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Two-photon Absorption and Nonlinear Optical Properties of A New Organic Dye DEASPI
Author(s): Guangyong Zhou, Xiaomei WANG, Dong Wang, Chun WANG, Xian ZHAO, Zongshu SHAO, Minhua JIANG
Pages: S139-
S142
Year: 2001
Issue:
z1
Journal: JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
Abstract: A new organic dye trans-4- [p-(N,N-diethylamino) styryl ]-N-methylpyridinium iodide (abbreviatedas DEASPI thereafter) with large two-photon absorption (TPA) cross section and excellent upconverted lasing properties was synthesized. The melting point and decompound point were measured to be 230℃ and 264.7℃ respectively. The molecular TPA cross section was meaThe linear and nonlinear optical properties of this dye were systematically studied. The highest net upconversion efficiency from the absorbed pump energy to the output upconverted lasing energy is as high as 18.6% at the pump energy of 2.17 mJ from a mode-locked Nd:YAG ps laser.The nonlinear transmittance at the wavelengths from 720 to 1100 nm was measured. The dye solution also shows a clear optical power limiting effect.
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