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Issue:
Hierarchical Equations of Motion for Quantum Dissipation and Quantum Transport
Author(s):
Zheng Xiao1 Xu Ruixue1 Xu Jian2 Jin Jinshuang3 Hu Jie2
,
4 Yan Yijing1
,
2*
Pages:
1129
-
1152
Year:
2012
Issue:
6
Journal:
Progress in Chemistry
Keyword:
量子耗散
;
量子输运
;
开放体系
;
级联方程组
;
Abstract:
级联方程已成为研究量子开放系统的稳态性质和动力学过程的重要方法。本文旨在系统综述量子耗散和量子输运的级联方程组方法的建立、发展以及在理论、算法和应用方面的一些最新进展。级联方程形式理论的建立以影响泛函路径积分为基础,并具有数值上的高效性和应用上的灵活性,可用于研究分子体系的复杂动力学过程以及强关联电子体系中的量子输运。其级联耦合结构以非微扰的方式揭示了多体相互作用、体系-环境耦合、非马尔可夫记忆等的综合效应。作为应用示例,我们采用级联方程模拟了生物光富集体系的二维相干动力学光谱以及含时电子输运过程中的动态近藤效应。
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